Free organic solvent ink containing graphite, carboxymethyl cellulose and microfibrillated cellulose as active material, dispersing and binder, respectively, has been formulated to produce flexible and eco-sustainable electrodes for lithium ion batteries. Content ratio of components and dispersion protocol were tailored in order to have rheological properties suitable for a large and cheap manufacturing process as well as screen printing. The bio-sourced printed electrodes exhibit a high porosity value of 70% that limits the electrochemical performances. However, the calendering process enhances electrode performances by increasing the reversible capacity from 85 until 315 mAh/g and reducing porosity to an optimal value of 34%. Moreover the introduction of 2% w/w of monofluoro-ethylene carbonate in the electrolyte reduced their reversible capacity loss of 11% in the printed electrode.